In order to realize electrostatic Stark deceleration of CH radicals and study cold chemistry, the fifth harmonic of a YAG laser is used to prepare CH (A2△) molecules through using the multi-photon dissociation of (CH3)eCO, CH3NO2, CHzBr2, and CHBr3 at ~ 213 nm. The CH product intensity is measured by using the emission spectrum of CH (A2△→XeH). The dependence of fluorescence intensity on laser power is studied, and the probable dissociation channels are analyzed. The relationship between the fluorescence intensity and some parameters, such as the temperature of the beam source, stagnation pressure, and the time delay between the opening of pulse valve and the photolysis laser, are also studied. The influence of three different carrier gases on CH signal intensity is investigated. The vibrational and rotational temperatures of the CH (Ae△) product are obtained by comparing experimental data with the simulated ones from the LIFBASE program.
By using the dispersion theory instead of the Frohlich Hamiltonian, the polaron energy in a quantum aot with a parabolic confinement potential is investigated at finite temperatures. It is found that the self-trapping energy of the polaron decreases with the increasing temperature, and the temperature effect is more obvious in quantum dots with weaker confinement.
This paper proposes a scheme of axial triple-well optical dipole trap by employing a simple optical system composed of a circular cosine grating and a lens. Three optical wells separated averagely by -37 μm were created when illuminating by a YAG laser with power 1 mW. These wells with average trapping depth -0.5 μK and volume -74 μm^3 are suitable to trap and manipulate an atomic Bose-Einstein condensation (BEC). Due to a controllable grating implemented by a spatial light modulator, an evolution between a triple-well trap and a single-well one is achievable by adjusting the height of potential barrier between adjacent wells. Based on this novel triple-well potentials, the loading and splitting of BEC, as well as the interference between three freely expanding BECs, are also numerically stimulated within the framework of mean-field treatment. By fitting three cosine functions with three Gaussian envelopes to interference fringe, the information of relative phases among three condensates is extracted.
Femtosecond coherent anti-Stokes Raman scattering (CARS) suffers from poor selectivity between neighbouring Raman levels due to the large bandwidth of the femtosecond pulses. This paper provides a new method to realize the selective excitation and suppression of femtosecond CARS by manipulating both the probe and pump (or Stokes) spectra. These theoretical results indicate that the CARS signals between neighbouring Raman levels are differentiated from their indistinguishable femtosecond CARS spectra by tailoring the probe spectrum, and then their selective excitation and suppression can be realized by supplementally manipulating the pump (or Stokes) spectrum with the π spectral phase step.